Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Graphene-assisted construction of electrocatalysts for carbon dioxide reduction | |
| Hu, Huawen1; Ou, Jian Zhen1,2; Xu, Xuejun1; Lin, Yinlei1; Zhang, Yuyuan1; Zhao, Hong1; Chen, Dongchu1; He, Minghui3; Huang, Yugang4,5; Deng, Lifang6 | |
| 2021-12-01 | |
| Source Publication | CHEMICAL ENGINEERING JOURNAL
 |
| ISSN | 1385-8947 |
| Volume | 425Pages:26 |
| Corresponding Author | Ou, Jian Zhen(Jianzhen.ou@rmit.edu.au) |
| Abstract | The electrochemical conversion of the greenhouse gas, carbon dioxide (CO2), to energy fuels and value-added chemicals presents one of the most valuable approaches to harvest pollutants and produce renewable energy. However, the stable molecular structure of CO2 and the sluggish reaction kinetics make CO2 reduction reaction (CO2RR) formidably challenging to achieve reaction rate and selectivity practical in industry. Graphene and its derivatives have been considered a group of intriguing materials to develop advanced CO2RR electrocatalysts due to their large specific surface area, remarkable electron transfer ability, superior stability, and easy tunability of the structure and surface properties. Herein, we comprehensively discuss the state-of-the-art electrocatalysts constructed with graphene and derivatives for active and selective CO2RR within the recent five years, mainly including the electrocatalysts with both metal-based (e.g., noble, non-noble, or combined thereof) and non-metal (e.g., doped, modified, defected, or composited) catalytic sites. To present the versatile, high-performance metal-based CO2RR electrocatalysts constructed with graphene, we further subdivide them according to the sizes, oxidation states, metal species synergies, dimensionalities, and versatility. Finally, we provide the challenges and perspectives in this emerging area of utilising CO2 to produce various carbon-based fuels and chemicals via graphene chemistry. |
| Keyword | Graphene Electrocatalysts CO2 reduction Metal-based Non-metal Active sites |
| DOI | 10.1016/j.cej.2021.130587 |
| WOS Keyword | NITROGEN-DOPED GRAPHENE ; EFFICIENT ELECTROCHEMICAL REDUCTION ; CO2 ELECTROREDUCTION PERFORMANCE ; METAL-FREE ELECTROCATALYST ; SINGLE-ATOM CATALYSTS ; OXYGEN REDUCTION ; SELECTIVE ELECTROREDUCTION ; FORMIC-ACID ; OXIDE ; NANOPARTICLES |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | Key-Area Special Project of Guangdong Provincial Education Department[2020ZDZX2066] ; Key Project of Guangdong Basic and Applied Basic Research Foundation[2020B1515120081] ; National Natural Science Foundation of China[51906045] ; National Natural Science Foundation of China[51803028] ; Key-Area Research and Development Program Project of Guangdong Province[2020B0909040002] ; National Natural Science Foundation of Guangdong Province[2019A1515010928] |
| WOS Research Area | Engineering |
| Funding Organization | Key-Area Special Project of Guangdong Provincial Education Department ; Key Project of Guangdong Basic and Applied Basic Research Foundation ; National Natural Science Foundation of China ; Key-Area Research and Development Program Project of Guangdong Province ; National Natural Science Foundation of Guangdong Province |
| WOS Subject | Engineering, Environmental ; Engineering, Chemical |
| WOS ID | WOS:000707126000064 |
| Publisher | ELSEVIER SCIENCE SA |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/35386 |
| Collection | 中国科学院广州能源研究所 |
| Corresponding Author | Ou, Jian Zhen |
| Affiliation | 1.Foshan Univ, Sch Mat Sci & Hydrogen Energy, Foshan 528000, Guangdong, Peoples R China 2.RMIT Univ, Sch Engn, Melbourne, Vic 3000, Australia 3.South China Univ Technol, Sch Light Ind & Engn, State Key Lab Pulp & Paper Engn, Guangzhou 510640, Guangdong, Peoples R China 4.Guangzhou Med Univ, Key Lab Mol Target & Clin Pharmacol, Guangzhou 511436, Guangdong, Peoples R China 5.Guangzhou Med Univ, Sch Pharmaceut Sci, Guangzhou 511436, Guangdong, Peoples R China 6.Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China |
| Recommended Citation GB/T 7714 | Hu, Huawen,Ou, Jian Zhen,Xu, Xuejun,et al. Graphene-assisted construction of electrocatalysts for carbon dioxide reduction[J]. CHEMICAL ENGINEERING JOURNAL,2021,425:26. |
| APA | Hu, Huawen.,Ou, Jian Zhen.,Xu, Xuejun.,Lin, Yinlei.,Zhang, Yuyuan.,...&Deng, Lifang.(2021).Graphene-assisted construction of electrocatalysts for carbon dioxide reduction.CHEMICAL ENGINEERING JOURNAL,425,26. |
| MLA | Hu, Huawen,et al."Graphene-assisted construction of electrocatalysts for carbon dioxide reduction".CHEMICAL ENGINEERING JOURNAL 425(2021):26. |
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