Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation | |
Li, Ming1,2,3; Fu, Junying1,2,3; Lv, Pengmei1,2,3,5 ; Zhang, Xufeng1,2,3; Liu, Xiaochun1,2,3,4; Zeng, Qiongyao1,2,3,4; Yang, Lingmei1,2,3; Wang, Zhongming1,2,3; Yuan, Zhenhong1,2,3
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| 2020-10-19 | |
| Source Publication | ACS SUSTAINABLE CHEMISTRY & ENGINEERING
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| ISSN | 2168-0485 |
| Volume | 8Issue:41Pages:15484-15495 |
| Corresponding Author | Fu, Junying(fujy@ms.giec.ac.cn) ; Lv, Pengmei(lvpm@ms.giec.ac.cn) |
| Abstract | Graphene-encapsulated nickel nanoparticles (Ni@C) were loaded on Zeolite Socony Mobil (ZSM)-5 for lipid hydrogenation to produce biojet fuel. Ni@C and ZSM-5 exhibit an efficient and synergistic catalytic activity, and the strong chemical interaction between graphene and nickel significantly improves the hydrogenation capacity of the catalyst. The graphene layers strengthened the dispersion of nickel, reduced the size of Ni@C to similar to 3.6 nm, and kept the valence state of nickel at 0. According to the hydrogenation tests, the conversion of oleic acid to jet fuel could reach 98.59% with only 3 wt % nickel loading amount. Furthermore, Ni@C/ZSM-5 shows excellent resistance to nickel agglomeration and loss. |
| Keyword | graphene hydrogenation jet fuel nickel loss nickel agglomeration |
| DOI | 10.1021/acssuschemeng.0c03559 |
| WOS Keyword | BIO-JET FUEL ; CARBON NANOTUBES ; FATTY-ACIDS ; OLEIC-ACID ; RANGE HYDROCARBONS ; VEGETABLE-OILS ; NONEDIBLE OIL ; FOSSIL-FUELS ; METAL ; CATALYSTS |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | Guangdong Special Support Program[2017TX04Z109] ; National Key RD Program[2019YFB1504003] ; Natural Science Foundation of Guangdong Province[2016A030308004] ; Natural Science Foundation of Guangdong Province[2018A030310078] ; National Natural Science Foundation of China[51861145103] ; National Natural Science Foundation of China Youth[51903236] |
| WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Engineering |
| Funding Organization | Guangdong Special Support Program ; National Key RD Program ; Natural Science Foundation of Guangdong Province ; National Natural Science Foundation of China ; National Natural Science Foundation of China Youth |
| WOS Subject | Chemistry, Multidisciplinary ; Green & Sustainable Science & Technology ; Engineering, Chemical |
| WOS ID | WOS:000584349900008 |
| Publisher | AMER CHEMICAL SOC |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/34857 |
| Collection | 中国科学院广州能源研究所 |
| Corresponding Author | Fu, Junying; Lv, Pengmei |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Collaborat Innovat Ctr Biomass Energy, Zhengzhou 450002, Henan, Peoples R China |
| First Author Affilication | GuangZhou Institute of Energy Conversion,Chinese Academy of Sciences |
| Recommended Citation GB/T 7714 | Li, Ming,Fu, Junying,Lv, Pengmei,et al. ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2020,8(41):15484-15495. |
| APA | Li, Ming.,Fu, Junying.,Lv, Pengmei.,Zhang, Xufeng.,Liu, Xiaochun.,...&Yuan, Zhenhong.(2020).ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,8(41),15484-15495. |
| MLA | Li, Ming,et al."ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 8.41(2020):15484-15495. |
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