GIEC OpenIR
Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media
Zhang, Xuemin1,2,3; Li, Jinping1,2; Wang, Jiaxian1,2; Wu, Qingbai1,4; Wang, Yingmei1,2; Yao, Ze1,2
2021-01-22
Source PublicationINTERNATIONAL JOURNAL OF GREEN ENERGY
ISSN1543-5075
Pages10
Corresponding AuthorZhang, Xuemin(zxm2010lut@163.com)
AbstractGas hydrate-based technology is a promising method for solidifying and sequestrating of CO2 gas into stratum sediments to reduce anthropogenic CO2 emissions and realize the exploitation of natural gas hydrate in the permafrost regions. In order to clarify the formation characteristics of CO2 hydrate in the porous media under condition of below the freezing point, the experiments were conducted in the frozen quartz sands. And the formation rate, the conversion rate and the gas storage capacities for CO2 hydrate were investigated through experimental study in the porous media. The results showed that, under the same temperature and initial pressure conditions, the formation rate, the conversion rate, and the gas storage capacities of hydrate increased with the decrease of particle sizes of the frozen quartz sands. And the ice content of the frozen quartz sands played little influence on the formation rate and the conversion rate of hydrate at the same particle size. Furthermore, the average formation rate attained 0.000544 mol center dot h(-1) in porous media below the freezing point. The conversion rate of ice attained 70.14, 81.72, and 90.61% in the frozen quartz sands with particle sizes of 500, 380, and 250 mu m, respectively. The results also illustrated that, the gas-storage capacity of hydrate achieved 127.58, 144.04, and 152.65 L/L in the corresponding porous media. These results are of signi?cance for guiding capture and sequestration of CO2 gas in the form of gas hydrate in stratum sediments.
KeywordGas hydrate porous media CO2 sequestration formation characteristics freezing point
DOI10.1080/15435075.2021.1875473
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[E029kf1501]
WOS Research AreaThermodynamics ; Science & Technology - Other Topics ; Energy & Fuels
Funding OrganizationNational Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences
WOS SubjectThermodynamics ; Green & Sustainable Science & Technology ; Energy & Fuels
WOS IDWOS:000619743900001
PublisherTAYLOR & FRANCIS INC
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/32687
Collection中国科学院广州能源研究所
Corresponding AuthorZhang, Xuemin
Affiliation1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou, Peoples R China
2.Key Lab Complementary Energy Syst Biomass & Solar, Lanzhou, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou, Peoples R China
4.Chinese Acad Sci, Cold & Arid Reg Environm & Engn Res Inst, State Key Lab Frozen Soil Engn, Lanzhou, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhang, Xuemin,Li, Jinping,Wang, Jiaxian,et al. Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media[J]. INTERNATIONAL JOURNAL OF GREEN ENERGY,2021:10.
APA Zhang, Xuemin,Li, Jinping,Wang, Jiaxian,Wu, Qingbai,Wang, Yingmei,&Yao, Ze.(2021).Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media.INTERNATIONAL JOURNAL OF GREEN ENERGY,10.
MLA Zhang, Xuemin,et al."Experimental study on formation characteristics of carbon dioxide hydrate in frozen porous media".INTERNATIONAL JOURNAL OF GREEN ENERGY (2021):10.
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