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Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions
Shan, Rui1,2,3,4; Lu, Lili1,2,3; Gu, Jing1,2,3,4; Zhang, Yuyuan5; Yuan, Haoran1,2,3,4; Chen, Yong1,2,3,4; Luo, Bo6
2020-08-01
Source PublicationMATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING
ISSN1369-8001
Volume114Pages:12
Corresponding AuthorYuan, Haoran(yuanhr@ms.giec.ac.cn)
AbstractOne set of biochar-coupled Ag and TiO2 composites were successfully fabricated by mixing, calcination, and photodeposition method to remove methyl orange (MO). It was found that all catalysts modified with Ag showed better photocatalytic degradation performance (the highest decolorization efficiency and mineralization efficiency were 97.48% and 85.38%, respectively) than single TiO2 because of the synergy of Ag, TiO2 and biochar. Characterization results indicated that Ag as well as TiO2 acted as electron donor and biochar acted as electron acceptor, which could effectively promote the separation of photogenerated electron hole pairs. In addition, the catalyst exhibited high stability up to 5 cycles and the loss of activity was negligible. And the catalytic degradation process was consistent with the pseudo-first-order kinetic (PFOK) model with the degradation rate constant of 6.29 x 10(2) min(-1).
KeywordAg Surface plasmon resonance Photocatalytic degradation Methyl orange TiO2
DOI10.1016/j.mssp.2020.105088
WOS KeywordVISIBLE-LIGHT ; ASSISTED SYNTHESIS ; TIO2 ; AG/TIO2 ; AG ; AG-TIO2 ; NANOCOMPOSITE ; NANOPARTICLES ; EFFICIENCY ; REDUCTION
Indexed BySCI
Language英语
Funding ProjectNational Key R&D Program of China[2018YFC1901200] ; National Natural Science Funds of China[51776211] ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China[GML2019ZD0101]
WOS Research AreaEngineering ; Materials Science ; Physics
Funding OrganizationNational Key R&D Program of China ; National Natural Science Funds of China ; Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou), China
WOS SubjectEngineering, Electrical & Electronic ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000535462600021
PublisherELSEVIER SCI LTD
Citation statistics
Cited Times:102[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/27119
Collection中国科学院广州能源研究所
Corresponding AuthorYuan, Haoran
Affiliation1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
2.Southern Marine Sci & Engn Guangdong Lab Guangzho, Guangzhou 511458, Peoples R China
3.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
4.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
5.Foshan Univ, Coll Mat Sci & Energy Engn, Foshan 528000, Guangdong, Peoples R China
6.Chongqing Environm & Sanitat Grp Co Ltd, Chongqing 401121, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Shan, Rui,Lu, Lili,Gu, Jing,et al. Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions[J]. MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING,2020,114:12.
APA Shan, Rui.,Lu, Lili.,Gu, Jing.,Zhang, Yuyuan.,Yuan, Haoran.,...&Luo, Bo.(2020).Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions.MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING,114,12.
MLA Shan, Rui,et al."Photocatalytic degradation of methyl orange by Ag/TiO2/biochar composite catalysts in aqueous solutions".MATERIALS SCIENCE IN SEMICONDUCTOR PROCESSING 114(2020):12.
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