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Effect of Initial Pressure on the Formation of Carbon Dioxide Hydrate in Frozen Quartz Sand
Zhang, Xuemin1,2; Li, Jinping1,2; Wu, Qingbai1,3; Wang, Yingmei1,2; Wang, Jiaxian1,2; Li, Yang1,2
2019-11-01
Source PublicationENERGY & FUELS
ISSN0887-0624
Volume33Issue:11Pages:11346-11352
Corresponding AuthorZhang, Xuemin(zxm2010lut@163.com)
AbstractSequestration and storage of CO2 in naturally occurring gas hydrate reservoirs is considered an effective strategy against global warming. In order to study the formation process of CO2 hydrate simulating the permafrost environment, the experiment was carried out in high-pressure vessel frozen quartz sand. The formation characteristics of CO2 hydrate were studied, and the influence of initial pressure on the hydrate formation process was discussed through experiments. The results showed that the formation rate of CO2 hydrate increased with the increase of the initial pressure of CO2 under the condition below the liquefied pressure. Furthermore, the formation rate of hydrate presented a similar change trend under the condition of the liquefied pressure. The results also indicated that the higher the initial pressure of CO2, the higher the final conversion rate of hydrate. Under the condition below the liquefied pressure, the highest conversion rate of ice was 66.3%. Furthermore, the highest conversion rate of ice attained 72.8% under the condition of the liquefied pressure. These results will provide a theoretical guidance for sequestration and storage of CO2 gas and exploitation of natural gas hydrate in permafrost regions.
DOI10.1021/acs.energyfuels.9b01693
WOS KeywordGAS HYDRATE ; METHANE HYDRATE ; POROUS-MEDIA ; DISSOCIATION ; EQUILIBRIUM ; CO2 ; CRYSTALLIZATION ; TEMPERATURES ; PARTICLES ; STABILITY
Indexed BySCI
Language英语
Funding ProjectNational Natural Science Foundation of China[51906093] ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences[Y907ke1001] ; Higher Education Innovative Ability Enhancement Project of Gansu Province[2019A-019] ; Hongliu Excellent Young Talents Support Program of Lanzhou University of Technology (2018)
WOS Research AreaEnergy & Fuels ; Engineering
Funding OrganizationNational Natural Science Foundation of China ; Open Fund of Key Laboratory of Gas Hydrate, Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences ; Higher Education Innovative Ability Enhancement Project of Gansu Province ; Hongliu Excellent Young Talents Support Program of Lanzhou University of Technology (2018)
WOS SubjectEnergy & Fuels ; Engineering, Chemical
WOS IDWOS:000499741900093
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:11[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.giec.ac.cn/handle/344007/25896
Collection中国科学院广州能源研究所
Corresponding AuthorZhang, Xuemin
Affiliation1.Lanzhou Univ Technol, Western China Res Ctr Energy & Environm, Lanzhou 730050, Gansu, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Northwest Inst Ecoenvironm & Resources, State Key Lab Frozen Soil Engn, Lanzhou 730000, Gansu, Peoples R China
First Author AffilicationGuangZhou Institute of Energy Conversion,Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Zhang, Xuemin,Li, Jinping,Wu, Qingbai,et al. Effect of Initial Pressure on the Formation of Carbon Dioxide Hydrate in Frozen Quartz Sand[J]. ENERGY & FUELS,2019,33(11):11346-11352.
APA Zhang, Xuemin,Li, Jinping,Wu, Qingbai,Wang, Yingmei,Wang, Jiaxian,&Li, Yang.(2019).Effect of Initial Pressure on the Formation of Carbon Dioxide Hydrate in Frozen Quartz Sand.ENERGY & FUELS,33(11),11346-11352.
MLA Zhang, Xuemin,et al."Effect of Initial Pressure on the Formation of Carbon Dioxide Hydrate in Frozen Quartz Sand".ENERGY & FUELS 33.11(2019):11346-11352.
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