Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method | |
Mei, Qun1,2; Wei, Xiangqian1; Sun, Weitao1; Zhang, Xinghua2; Li, Wenzhi1; Ma, Longlong2 | |
2019 | |
发表期刊 | RSC ADVANCES |
ISSN | 2046-2069 |
卷号 | 9期号:23页码:12846-12853 |
通讯作者 | Li, Wenzhi(liwenzhi@ustc.edu.cn) ; Ma, Longlong(mall@ms.giec.ac.cn) |
摘要 | Conversion of cellulose to 5-hydroxymethylfurfural (HMF) is an important means of biomass utilization. However, simulation of hydrolysis of cellulose and species transport in multiphase systems is still missing. In this paper, a multiphase lattice Boltzmann method of the Shan-Chen model has been applied for simulating the complex chemical reactions and interphase mass transfer in a liquid membrane catalytic reactor. For the sake of simplification, a single particle liquid membrane catalytic model is developed to simulate the hydrolysis of cellulose into HMF and its side reactions, which include the adsorption of cellulose particles on the liquid membrane, the complex chemical reactions inside the liquid membrane and the interphase transfer of HMF. This simulation presents the results of hydrolysis of cellulose and the HMF transport process. Additionally, the results show that the thinner liquid membrane thickness is beneficial for increasing the yield of HMF. |
DOI | 10.1039/c9ra02090j |
关键词[WOS] | BIOMASS FAST PYROLYSIS ; MASS-TRANSFER ; SIMULATION ; DEHYDRATION ; CONVERSION ; FRUCTOSE ; ZEOLITE ; FLOW |
收录类别 | SCI |
语种 | 英语 |
资助项目 | National Natural Science Foundation of China[51576198] ; National Natural Science Foundation of China[51536009] ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21060102] |
WOS研究方向 | Chemistry |
项目资助者 | National Natural Science Foundation of China ; Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences |
WOS类目 | Chemistry, Multidisciplinary |
WOS记录号 | WOS:000468636000008 |
出版者 | ROYAL SOC CHEMISTRY |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.giec.ac.cn/handle/344007/24979 |
专题 | 中国科学院广州能源研究所 |
通讯作者 | Li, Wenzhi; Ma, Longlong |
作者单位 | 1.Univ Sci & Technol China, Dept Thermal Sci & Energy Engn, Lab Basic Res Biomass Convers & Utilizat, Hefei 230026, Anhui, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, CAS Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China |
第一作者单位 | 中国科学院广州能源研究所 |
推荐引用方式 GB/T 7714 | Mei, Qun,Wei, Xiangqian,Sun, Weitao,et al. Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method[J]. RSC ADVANCES,2019,9(23):12846-12853. |
APA | Mei, Qun,Wei, Xiangqian,Sun, Weitao,Zhang, Xinghua,Li, Wenzhi,&Ma, Longlong.(2019).Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method.RSC ADVANCES,9(23),12846-12853. |
MLA | Mei, Qun,et al."Liquid membrane catalytic model of hydrolyzing cellulose into 5-hydroxymethylfurfural based on the lattice Boltzmann method".RSC ADVANCES 9.23(2019):12846-12853. |
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