Knowledge Management System Of Guangzhou Institute of Energy Conversion, CAS
| Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts | |
Guo, Haijun1,2; Zhang, Hairong1,2; Peng, Fen1,2; Yang, Huijuan1,2,3; Xiong, Lian1,2; Huang, Chao1,2; Wang, Can1,2; Chen, Xinde1,2 ; Ma, Longlong1,2
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| 2015-07-01 | |
| Source Publication | APPLIED CLAY SCIENCE
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| Volume | 111Pages:83-89 |
| Abstract | Conversion of lignocellulosic biomass to liquid fuels through the synthesis gas (syngas) intermediate product will become an important route for production of clean fuel in the future. In this work, H2SO4-activated palygorskite (Pal) supported Cu-Fe-Co based catalysts were prepared by an impregnation method and applied to mixed alcohols synthesis (MAS) from syngas. The structural properties of those catalysts were characterized by N-2 adsorption/desorption, X-ray diffraction (XRD), X-ray fluorescence (XRF), X-ray photoelectron spectroscopy (XPS), Scanning Electron Microscope (SEM), Transmission electron microscopy (TEM) and H-2-Temperature programmed reduction (H-2-TPR). The CFCK/Pal-B21 catalyst exhibited better catalytic activity, yield and selectivity for mixed alcohols due to the high surface concentration of Cu-FeCx dual site and the ideal interaction between Cu and Fe species. Due to the unique property and the low cost and easy availability, the Pal clay has a great promise to be used as catalyst support for liquid biofuel production from biomass-derived syngas. (C) 2015 Elsevier B.V. All rights reserved. |
| Subtype | Article |
| Keyword | Syngas Mixed Alcohols Synthesis Palygorskite Cu-fe-co Based Catalyst |
| WOS Headings | Science & Technology ; Physical Sciences ; Technology |
| DOI | 10.1016/j.clay.2015.03.009 |
| WOS Subject Extended | Chemistry ; Materials Science ; Mineralogy |
| WOS Keyword | BIMETALLIC NANOPARTICLES ; SURFACE-PROPERTIES ; ATTAPULGITE CLAY ; CONVERSION ; BIOMASS ; HYDROGENATION ; EVOLUTION ; OXIDATION ; KINETICS ; COPPER |
| Indexed By | SCI |
| Language | 英语 |
| WOS Subject | Chemistry, Physical ; Materials Science, Multidisciplinary ; Mineralogy |
| WOS ID | WOS:000355362600011 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.giec.ac.cn/handle/344007/10501 |
| Collection | 中国科学院广州能源研究所 集成技术研发中心 |
| Affiliation | 1.Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy, Guangzhou 510640, Guangdong, Peoples R China 2.Chinese Acad Sci, Guangzhou Inst Energy Convers, R&D Ctr Xuyi Attapulgite Appl Technol, Guangzhou 211700, Guangdong, Peoples R China 3.Chinese Acad Sci, Grad Univ, Being 100049, Peoples R China |
| Recommended Citation GB/T 7714 | Guo, Haijun,Zhang, Hairong,Peng, Fen,et al. Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts[J]. APPLIED CLAY SCIENCE,2015,111:83-89. |
| APA | Guo, Haijun.,Zhang, Hairong.,Peng, Fen.,Yang, Huijuan.,Xiong, Lian.,...&Ma, Longlong.(2015).Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts.APPLIED CLAY SCIENCE,111,83-89. |
| MLA | Guo, Haijun,et al."Mixed alcohols synthesis from syngas over activated palygorskite supported Cu-Fe-Co based catalysts".APPLIED CLAY SCIENCE 111(2015):83-89. |
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