Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge

doi:10.1016/j.apenergy.2012.12.017

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	Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge
	Ding, Mingyue1 ; Hayakawa, Taichi 2; Zeng, Chunyang 2; Jin, Yuzhou 2; Zhang, Qi1 ; Wang, Tiejun1 ; Ma, Longlong1 ; Yoneyama, Yoshiharu 2; Tsubaki, Noritatsu 2,3
	2013-04-01
Source Publication	APPLIED ENERGY
Volume	104 Pages:777-782
Abstract	Non-catalytic direct conversion of liquid natural gas (LNG) to syngas and ethylene using pulse discharge technology was firstly carried out under the temperature of liquid nitrogen and atmospheric pressure. The liquefaction of natural gas increased tremendously the collision frequency between electrons and methane molecules in the discharge region and promoted the dimerisation of CH2 radicals formed, inducing the formation of large amounts of ethylene (selectivity > 90%) and synthesis gas, and suppressing the proceeding of useless side-reactions. Especially, CO2 formation was suppressed remarkably due to the very low temperature of LNG and the cage effect provided by the condensed LNG. Crown Copyright (C) 2012 Published by Elsevier Ltd. All rights reserved.
Subtype	Article
Keyword	Liquid Natural Gas Pulse Discharge Technology Cage Effect Syngas And Ethylene
WOS Headings	Science & Technology ; Technology
DOI	10.1016/j.apenergy.2012.12.017
WOS Subject Extended	Energy & Fuels ; Engineering
WOS Keyword	CATALYTIC PARTIAL-OXIDATION ; LOW-TEMPERATURE PLASMA ; METHANE CONVERSION ; ATMOSPHERIC-PRESSURE ; ROOM-TEMPERATURE ; ACETYLENE ; ACTIVATION
Indexed By	SCI
Language	英语
WOS Subject	Energy & Fuels ; Engineering, Chemical
WOS ID	WOS:000316152700075
Citation statistics	Cited Times:11[WOS] [WOS Record] [Related Records in WOS]
Document Type	期刊论文
Identifier	http://ir.giec.ac.cn/handle/344007/10036
Collection	中国科学院广州能源研究所
Affiliation	1.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou 510640, Guangdong, Peoples R China 2.Toyama Univ, Dept Appl Chem, Sch Engn, Toyama 9308555, Japan 3.Japan Sci & Technol Agcy JST, ACT C, Tokyo 1028666, Japan
Recommended Citation GB/T 7714	Ding, Mingyue,Hayakawa, Taichi,Zeng, Chunyang,et al. Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge[J]. APPLIED ENERGY,2013,104:777-782.
APA	Ding, Mingyue.,Hayakawa, Taichi.,Zeng, Chunyang.,Jin, Yuzhou.,Zhang, Qi.,...&Tsubaki, Noritatsu.(2013).Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge.APPLIED ENERGY,104,777-782.
MLA	Ding, Mingyue,et al."Direct conversion of liquid natural gas (LNG) to syngas and ethylene using non-equilibrium pulsed discharge".APPLIED ENERGY 104(2013):777-782.

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